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Synthesis, crystal structure and Hirshfeld surface analysis of a zinc(II) coordination polymer of 5-phenyl-1,3,4-oxadiazole-2-thiolate

Мehribon PirimovaNational University of Uzbekistan named after Mirzo Ulugbek, 4 University St, Tashkent, 100174, UzbekistanBаtirbаy TоrаmbеtоvNational University of Uzbekistan named after Mirzo Ulugbek, 4 University St, Tashkent, 100174, UzbekistanShakhnoza KadirovaNational University of Uzbekistan named after Mirzo Ulugbek, 4 University St, Tashkent, 100174, UzbekistanA. A. ZiyaevS. Yu. Yunusov Institute of the Chemistry of Plant Substances, Academy of Sciences of the Republic of Uzbekistan, Mirzo Ulugbek Str. 77, 100170, Tashkent, UzbekistanRajesh G. GonnadePhysical and Materials Chemistry Division, CSIR-National Chemical Laboratory, Pune-411008, IndiaJamshid AshurovInstitute of Bioorganic Chemistry, Academy of Sciences of Uzbekistan, M. Ulugbek Str, 83, Tashkent, 100125, Uzbekistan
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Abstract

A new zinc coordination polymer with 5-phenyl-1,3,4-oxadiazole-2-thiolate, namely, catena -poly[zinc(II)-bis(μ 2 -5-phenyl-1,3,4-oxadiazole-2-thiolato)-κ 2 N 3 : S ;κ 2 S : N 3 ], [Zn(C 8 H 5 N 2 OS) 2 ] n , was synthesized. The single-crystal X-ray diffraction analysis shows that the polymeric structure crystallizes in the centrosymmetric monoclinic C 2/ c space group. The Zn II atom is coordinated to two S and two N atoms from four crystallographically independent ( L ) ligands, forming zigzag chains along the [001] direction. This polymer complex forms an eight-membered [Zn–S–C–N–Zn–S–C–N] chair-like ring with two Zn II atoms and two ligand molecules. On the Hirshfeld surface, the largest contributions come from the short contacts such as van der Waals forces, including H...H, C...H and S...H. Interactions including N...H, O...H and C...C contacts were also observed; however, their contribution to the overall stability of the crystal lattice is minor.

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