Boosting water decomposition by sulfur vacancies for efficient CO<sub>2</sub> photoreduction
Shikang YinInstitute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, P. R. ChinaXiaoxue ZhaoInstitute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, P. R. ChinaEnhui JiangInstitute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, P. R. ChinaPeng ZhouDepartment of Electrical Engineering and Computer Science, University of Michigan, Ann Arbor, MI 48109, USAPengwei HuoInstitute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, P. R. China
2022en
ABI
Abstract
As the rate-determining half reaction (OER) in the overall CO 2 photoreduction, the four-electron-involving OER on S-vacancy sites was favored, therefore facilitating the hole-elimination/proton release and unleashing the CO 2 reduction half reaction.
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