Attosecond nonlinear optics using gigawatt-scale isolated attosecond pulses
Abstract
High-energy isolated attosecond pulses required for the most intriguing nonlinear attosecond experiments as well as for attosecond-pump/attosecond-probe spectroscopy are still lacking at present. Here we propose and demonstrate a robust generation method of intense isolated attosecond pulses, which enable us to perform a nonlinear attosecond optics experiment. By combining a two-colour field synthesis and an energy-scaling method of high-order harmonic generation, the maximum pulse energy of the isolated attosecond pulse reaches as high as 1.3 μJ. The generated pulse with a duration of 500 as, as characterized by a nonlinear autocorrelation measurement, is the shortest and highest-energy pulse ever with the ability to induce nonlinear phenomena. The peak power of our tabletop light source reaches 2.6 GW, which even surpasses that of an extreme-ultraviolet free-electron laser. The short duration of attosecond pulses makes them interesting for ultrafast experiments, although it has so far been difficult to generate isolated attosecond pulses with sufficiently high power. Here the authors achieve high-intensity isolated attosecond pulses with a tabletop setup, based on a scaled-up high-order harmonic generation process.