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Charged-soliton dynamics in<i>trans</i>-polyacetylene

Lewis J. RothbergAT&T Bell Laboratories, Murray Hill, New Jersey 07974T. M. JedjuAT&T Bell Laboratories, Murray Hill, New Jersey 07974S. EtemadAT&T Bell Laboratories, Murray Hill, New Jersey 07974G. L. BakerAT&T Bell Laboratories, Murray Hill, New Jersey 07974
1986en
ABI

Abstract

Piscosecond time-resolved absorption studies of the midgap absorption associated with photogenerated charged solitons in trans-polyacetylene are reported. Both direct photogeneration of charged-soliton pairs and neutral- to charged-soliton conversion are observed. The former are created by intrachain absorption and decay on a subpicosecond time scale. The latter are formed following interchain photoexcitation and are the dominant population of charged solitons at times greater than 20 ps.

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