Magnons in the Linear-Chain Antiferromagnet CsMn<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">Cl</mml:mi></mml:mrow><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>·2<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">D</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>O
J. SkalyoBrookhaven National Laboratory, Upton, New York 11973G. ShiraneBrookhaven National Laboratory, Upton, New York 11973S. A. FriedbergBrookhaven National Laboratory, Upton, New York 11973H. KobayashiBrookhaven National Laboratory, Upton, New York 11973
1970lv
ABI
Abstract
This paper reports the first neutron scattering measurements on spin waves in a linear-chain antiferromagnet. Measurements were made on CsMn${\mathrm{Cl}}_{3}$\ifmmode\cdot\else\textperiodcentered\fi{}2${\mathrm{D}}_{2}$O and clearly indicate a large directional anisotropy of the spin coupling. The dominant exchange occurs along chains extending in the $a$ direction, ${J}_{1}=\ensuremath{-}0.304\ifmmode\pm\else\textpm\fi{}0.003$ meV. The exchange parameters in the $b$ and $c$ directions were measured in the combinative form ${J}_{2}+{J}_{3}=\ensuremath{-}0.0021\ifmmode\pm\else\textpm\fi{}0.0004$ meV. Short-wavelength excitations along the chain direction persist even at $2{T}_{N}$.
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