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Methylene Blue Dye Photocatalytic Degradation over Synthesised Fe3O4/AC/TiO2 Nano-Catalyst: Degradation and Reusability Studies

Seyedehmaryam MoosaviNanotechnology & Catalysis Research Centre (NANOCAT), Institute for Advanced Studies (IAS), University for Malaya (UM), Level 3, Block A, Kuala Lumpur 50603, MalaysiaRita Yi Man LiSustainable Real Estate Research Center, Hong Kong Shue Yan University, North Point, Hong Kong 999077Chin Wei LaiNanotechnology & Catalysis Research Centre (NANOCAT), Institute for Advanced Studies (IAS), University for Malaya (UM), Level 3, Block A, Kuala Lumpur 50603, MalaysiaYusliza YusofNanotechnology & Catalysis Research Centre (NANOCAT), Institute for Advanced Studies (IAS), University for Malaya (UM), Level 3, Block A, Kuala Lumpur 50603, MalaysiaSinyee GanPublication Unit, Information Technology and Corporate Services Division, Malaysian Palm Oil Board (MPOB), Kajang 43000, Selangor, MalaysiaOmid AkbarzadehNanotechnology & Catalysis Research Centre (NANOCAT), Institute for Advanced Studies (IAS), University for Malaya (UM), Level 3, Block A, Kuala Lumpur 50603, MalaysiaZaira Zaman ChowhuryNanotechnology & Catalysis Research Centre (NANOCAT), Institute for Advanced Studies (IAS), University for Malaya (UM), Level 3, Block A, Kuala Lumpur 50603, MalaysiaXiao‐Guang YueFaculty of Engineering and Technology, Siksha ‘O’ Anusandhan University, Bhubaneswar 751030, IndiaMohd RafieBin JohanNanotechnology & Catalysis Research Centre (NANOCAT), Institute for Advanced Studies (IAS), University for Malaya (UM), Level 3, Block A, Kuala Lumpur 50603, Malaysia
2020en
ABI

Аннотация

In this study, activated carbon (AC) from coconut shell, as a widely available agricultural waste, was synthesised in a simple one-step procedure and used to produce a magnetic Fe3O4/AC/TiO2 nano-catalyst for the degradation of methylene blue (MB) dye under UV light. Scanning electron microscopy revealed that TiO2 nanoparticles, with an average particle size of 45 to 62 nm, covered the surface of the AC porous structure without a reunion of its structure, which according to the TGA results enhanced the stability of the photocatalyst at high temperatures. The photocatalytic activities of synthesised AC, commercial TiO2, Fe3O4/AC, and Fe3O4/AC/TiO2 were compared, with Fe3O4/AC/TiO2 (1:2) exhibiting the highest catalytic activity (98%). Furthermore, evaluation of the recovery and reusability of the photocatalysts after treatment revealed that seven treatment cycles were possible without a significant reduction in the removal efficiency.

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