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Interface engineering of highly efficient perovskite solar cells

Huanping ZhouCalifornia NanoSystems Institute, University of California, Los Angeles, CA 90095, USAQi ChenCalifornia NanoSystems Institute, University of California, Los Angeles, CA 90095, USAGang LiDepartment of Materials Science and Engineering, University of California, Los Angeles, CA 90095, USASong LuoCalifornia NanoSystems Institute, University of California, Los Angeles, CA 90095, USATze‐Bin SongCalifornia NanoSystems Institute, University of California, Los Angeles, CA 90095, USAHsin‐Sheng DuanCalifornia NanoSystems Institute, University of California, Los Angeles, CA 90095, USAZiruo HongDepartment of Materials Science and Engineering, University of California, Los Angeles, CA 90095, USAJingbi YouDepartment of Materials Science and Engineering, University of California, Los Angeles, CA 90095, USAYongsheng LiuCalifornia NanoSystems Institute, University of California, Los Angeles, CA 90095, USAYang YangCalifornia NanoSystems Institute, University of California, Los Angeles, CA 90095, USA
2014en
ABI

Аннотация

Advancing perovskite solar cell technologies toward their theoretical power conversion efficiency (PCE) requires delicate control over the carrier dynamics throughout the entire device. By controlling the formation of the perovskite layer and careful choices of other materials, we suppressed carrier recombination in the absorber, facilitated carrier injection into the carrier transport layers, and maintained good carrier extraction at the electrodes. When measured via reverse bias scan, cell PCE is typically boosted to 16.6% on average, with the highest efficiency of ~19.3% in a planar geometry without antireflective coating. The fabrication of our perovskite solar cells was conducted in air and from solution at low temperatures, which should simplify manufacturing of large-area perovskite devices that are inexpensive and perform at high levels.

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