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Uniform and staggered magnetizations induced by Dzyaloshinskii-Moriya interactions in isolated and coupled spin-<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:mn>1</mml:mn><mml:mo>∕</mml:mo><mml:mn>2</mml:mn></mml:mrow></mml:math>dimers in a magnetic field

Shin MiyaharaDepartment of Physics and Mathematics, Aoyama Gakuin University, Sagamihara, Kanagawa 229-8558, JapanJ.-B. FouetSalvatore R. ManmanaFachbereich Physik, Philipps Universität Marburg, D-35032 Marburg, GermanyR. M. NoackFachbereich Physik, Philipps Universität Marburg, D-35032 Marburg, GermanyH. MayaffreLaboratoire de Spectrométrie Physique, Université J. Fourier & UMR5588 CNRS, BP 87, 38402 Saint Martin d’Hères, FranceI. SheikinGrenoble High Magnetic Field Laboratory, CNRS, BP 166, F-38042 Grenoble Cedex 09, FranceC. BerthierGrenoble High Magnetic Field Laboratory, CNRS, BP 166, F-38042 Grenoble Cedex 09, FranceFrédéric MilaInstitute of Theoretical Physics, École Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland
2007lv
ABI

Аннотация

We investigate the interplay of Dzyaloshinskii-Moriya interactions and an external field in spin-$1∕2$ dimers. For isolated dimers and at low field, we derive simple expressions for the staggered and uniform magnetizations which show that the orientation of the uniform magnetization can deviate significantly from that of the external field. In fact, in the limit where the $\mathbf{D}$ vector of the Dzyaloshinskii-Moriya interaction is parallel to the external field, the uniform magnetization actually becomes perpendicular to the field. For larger fields, we show that the staggered magnetization of an isolated dimer has a maximum close to one-half the polarization, with a large maximal value of $0.35g{\ensuremath{\mu}}_{B}$ in the limit of very small Dzyaloshinskii-Moriya interaction. We investigate the effect of interdimer coupling in the context of ladders with density-matrix renormalization-group (DMRG) calculations and show that, as long as the values of the Dzyaloshinskii-Moriya interaction and of the exchange interaction are compatible with respect to the development of a staggered magnetization, the simple picture that emerges for isolated dimers is also valid for weakly coupled dimers with minor modifications. The results are compared with torque measurements on ${\mathrm{Cu}}_{2}{({\mathrm{C}}_{5}{\mathrm{H}}_{12}{\mathrm{N}}_{2})}_{2}{\mathrm{Cl}}_{4}$.

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