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Dissolution swelling effect-assisted interfacial morphology refinement enables high efficiency all-polymer solar cells

Weichao ZhangCAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, P. R. ChinaYaochang YueSchool of Chemistry, Beijing Advanced Innovation Center for Biomedical Engineering, Beihang University, Beijing 100191, P. R. ChinaFei HanFrontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaHong ZhangCAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, P. R. ChinaYongqing WangSchool of Chemistry, Beijing Advanced Innovation Center for Biomedical Engineering, Beihang University, Beijing 100191, P. R. ChinaShengli YueSchool of Chemistry, Beijing Advanced Innovation Center for Biomedical Engineering, Beihang University, Beijing 100191, P. R. ChinaBohao SongFrontier Institute of Science and Technology, Xi’an Jiaotong University, Xi’an, 710054, ChinaGuanghan ZhaoCAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, P. R. ChinaChao QuSchool of Chemistry, Beijing Advanced Innovation Center for Biomedical Engineering, Beihang University, Beijing 100191, P. R. ChinaRongsheng YangSchool of Chemistry, Beijing Advanced Innovation Center for Biomedical Engineering, Beihang University, Beijing 100191, P. R. ChinaRui ZengFrontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaShilin LiSchool of Chemistry, Beijing Advanced Innovation Center for Biomedical Engineering, Beihang University, Beijing 100191, P. R. ChinaChuanyun LiCAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, P. R. ChinaJin ZhouCAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, P. R. ChinaGuanghao LuFrontier Institute of Science and Technology, Xi’an Jiaotong University, Xi’an, 710054, ChinaWanfei ShiCAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, P. R. ChinaXuning ZhangCollege of Physics Science & Technology, Hebei University, Hebei, 071000, ChinaFeng LiuFrontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaMing ZhangFrontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaHuiqiong ZhouCAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, P. R. ChinaYuan ZhangSchool of Chemistry, Beijing Advanced Innovation Center for Biomedical Engineering, Beihang University, Beijing 100191, P. R. China
2024en
ABI

Аннотация

Small molecule incorporation during sequential deposition improved donor crystallization and intercalation, optimizing the heterojunction morphology. The PCEs achieved 19.39% for small-area (0.04 cm 2 ) and 17.71% for large-area (1 cm 2 ) devices.

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