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Mechanosynthesized electroactive materials for sustainable energy and environmental applications: A critical review

Zhijie ChenSchool of Civil and Environmental Engineering, University of New South Wales, Sydney, NSW 2052, AustraliaGao‐Feng HanKey Laboratory of Automobile Materials, Ministry of Education, and School of Materials Science and Engineering, Jilin University, Changchun, PR ChinaAsif MahmoodCentre for Clean Energy Technology, School of Mathematical and Physical Sciences, Faculty of Science, University of Technology Sydney, City Campus, Broadway, NSW 2007, AustraliaJingwei HouSchool of Chemical Engineering, University of Queensland, Queensland 4072, AustraliaWei WeiCentre for Technology in Water and Wastewater, School of Civil and Environmental Engineering, University of Technology Sydney, NSW 2007, AustraliaHo Kyong ShonCentre for Technology in Water and Wastewater, School of Civil and Environmental Engineering, University of Technology Sydney, NSW 2007, AustraliaGuoxiu WangCentre for Clean Energy Technology, School of Mathematical and Physical Sciences, Faculty of Science, University of Technology Sydney, City Campus, Broadway, NSW 2007, AustraliaT. David WaiteSchool of Civil and Environmental Engineering, University of New South Wales, Sydney, NSW 2052, AustraliaJong‐Beom BaekSchool of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks, Ulsan National Institute of Science and Technology (UNIST), 50 UNIST, Ulsan 44919, South KoreaBing‐Jie NiSchool of Civil and Environmental Engineering, University of New South Wales, Sydney, NSW 2052, Australia
2024en
ABI

Аннотация

Electrochemistry-driven techniques for advanced energy storage/conversion and environmental protection play a crucial role in achieving sustainable development goals. As an indispensable component in diverse electrochemical systems, electroactive materials gain soaring interest in terms of rational design and sustainable synthesis. Notably, mechanochemistry-based green and powerful synthesis has been widely employed to fabricate diverse electroactive materials, given their scalability and tunability. Recently, mechanochemically synthesized electroactive materials have been widely applied in various environmental and energy fields, leading to significant progress. However, a systematic analysis of these advancements is still missing. Herein, we comprehensively discuss recent achievements in mechanosynthesized electroactive materials for sustainable energy and environmental applications. The development of mechanochemical synthesis is introduced, along with different types of mechanosynthesized electroactive materials. Subsequently, the review delves into the applications of these materials in advanced energy conversion/storage systems and environmental remediation. The rational design of electroactive materials and their structure-performance correlation are illustrated by discussing the effects of the mechanochemical process on the internal and external properties of materials and their electrochemical performance. Lastly, key perspectives in this field are discussed, including mechanochemical process monitoring, field-assisted mechanochemical synthesis, material performance optimization, practical applications, and mechanochemistry-driven fuels/chemicals synthesis. By illustrating current advances and perspectives related to the development of mechanosynthesized electroactive materials, this review aims to shed some light on upcoming research on green mechanochemical synthesis-driven energy and environmental sustainability.

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