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Toward Flexible and Stretchable Organic Solar Cells: A Comprehensive Review of Transparent Conductive Electrodes, Photoactive Materials, and Device Performance

Yong YanCo‐Innovation Center of Efficient Processing and Utilization of Forest Resources College of Materials Science and Engineering Nanjing Forestry University Nanjing 210037 ChinaBowen DuanCo‐Innovation Center of Efficient Processing and Utilization of Forest Resources College of Materials Science and Engineering Nanjing Forestry University Nanjing 210037 ChinaMin RuCo‐Innovation Center of Efficient Processing and Utilization of Forest Resources College of Materials Science and Engineering Nanjing Forestry University Nanjing 210037 ChinaQilin GuCo‐Innovation Center of Efficient Processing and Utilization of Forest Resources College of Materials Science and Engineering Nanjing Forestry University Nanjing 210037 ChinaSunsun LiKey Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM) Nanjing Tech University (NanjingTech) Nanjing Jiangsu 211816 ChinaWenchao ZhaoCo‐Innovation Center of Efficient Processing and Utilization of Forest Resources College of Materials Science and Engineering Nanjing Forestry University Nanjing 210037 China
2024en
ABI

Аннотация

Abstract Flexible and stretchable organic solar cells (FOSCs and SOSCs) hold immense potential due to their versatility and applicability in emerging areas such as wearable electronics, foldable devices, and biointegrated systems. Despite these promising applications, several challenges remain, primarily related to the mechanical durability, material performance, and scalability required for commercialization. This review comprehensively highlights recent advancements in the design and fabrication of FOSCs and SOSCs, with a particular emphasis on key functional layers, including transparent conductive electrodes, interfacial layers, photoactive materials, and top electrodes. Innovations in material design, such as active layers and transparent conductive electrodes with improved flexibility, are discussed alongside developments in device processes to achieve power conversion efficiencies exceeding 19%. Furthermore, the review addresses remaining challenges, including the need for scalable manufacturing techniques and enhanced mechanical robustness under strain. Finally, the prospects of FOSCs and SOSCs are analyzed, providing insights into how these technologies can contribute to the development of sustainable, high‐performance power sources for wearable electronic devices and other flexible electronics. This review offers valuable insights, bringing the commercialization of wearable, high‐performance FOSCs and SOSCs closer to reality.

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