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Experiments on the synthesis of superheavy nuclei<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mmultiscripts><mml:mi>Fl</mml:mi><mml:mprescripts/><mml:none/><mml:mn>284</mml:mn></mml:mmultiscripts></mml:math>and<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mmultiscripts><mml:mi>Fl</mml:mi><mml:mprescripts/><mml:none/><mml:mn>285</mml:mn></mml:mmultiscripts></mml:math>in the<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mmultiscripts><mml:mi>Pu</mml:mi><mml:mprescripts/><mml:none/><mml:mrow><mml:mn>239</mml:mn><mml:mo>,</mml:mo><mml:mn>240</mml:mn></mml:mrow></mml:mmultiscripts><mml:mo>+</mml:mo><mml:mmultiscripts><mml:mi>Ca</mml:mi><mml:mprescripts/><mml:none/><mml:mn>48</mml:mn></mml:mmultiscripts></mml:mrow></mml:math>reactions

V. K. UtyonkovFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationN. T. BrewerPhysics Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USAYu. Ts. OganessianFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationKonrad RykaczewskiPhysics Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USAF. Sh. AbdullinFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationS. N. DmitrievFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationR. GrzywaczDepartment of Physics and Astronomy, University of Tennessee, Knoxville, Tennessee 37996, USAМ. Г. ИткисFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationK. MiernikFaculty of Physics, University of Warsaw, PL-02-093 Warsaw, PolandA. N. PolyakovFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationJ. B. RobertoScience and Technology Partnerships Directorate, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USAR. N. SagaidakFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationI. V. ShirokovskyFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationM. V. ShumeikoFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationYu. S. TsyganovFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationA. A. VoinovFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationV. G. SubbotinFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationA. M. SukhovFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationA. V. SabelnikovFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationG. K. VostokinFlerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research, RU-141980 Dubna, Russian FederationJ. H. HamiltonDepartment of Physics and Astronomy, Vanderbilt University, Nashville, Tennessee 37235, USAM. A. StoyerNuclear and Chemical Sciences Division, Lawrence Livermore National Laboratory, Livermore, California 94551, USAS. StraussDepartment of Physics, University of Notre Dame, Notre Dame, Indiana 46566, USA
2015lv
ABI

Аннотация

Irradiations of $^{239}\mathrm{Pu}$ and $^{240}\mathrm{Pu}$ targets with $^{48}\mathrm{Ca}$ beams aimed at the synthesis of $Z=114$ flerovium isotopes were performed at the Dubna Gas Filled Recoil Separator. A new spontaneously fissioning (SF) isotope $^{284}\mathrm{Fl}$ was produced for the first time in the $^{240}\mathrm{Pu}+^{48}\mathrm{Ca}$ (250 MeV) and $^{239}\mathrm{Pu}+^{48}\mathrm{Ca}$ (245 MeV) reactions. The cross section of the $^{239}\mathrm{Pu}(^{48}\mathrm{Ca},3n)^{284}\mathrm{Fl}$ reaction channel was about 20 times lower than predicted by theoretical models and about 50 times lower than the maximum fusion-evaporation cross section for the $3n$ and $4n$ channels measured in the $^{244}\mathrm{Pu}+^{48}\mathrm{Ca}$ reaction. In the $^{240}\mathrm{Pu}+^{48}\mathrm{Ca}$ experiment, performed at 245 MeV in order to maximize the $3n$-evaporation channel, three decay chains of $^{285}\mathrm{Fl}$ were detected. The $\ensuremath{\alpha}$-decay energy of $^{285}\mathrm{Fl}$ was measured for the first time and decay properties of its descendants $^{281}\mathrm{Cn}, ^{277}\mathrm{Ds}, ^{273}\mathrm{Hs}, ^{269}\mathrm{Sg}$, and $^{265}\mathrm{Rf}$ were determined with higher accuracy. The assignment of SF events observed during the irradiation of the $^{240}\mathrm{Pu}$ target with a 250 MeV $^{48}\mathrm{Ca}$ beam to $^{284}\mathrm{Fl}$ decay is presented and discussed. The cross sections at both $^{48}\mathrm{Ca}$ energies are similar and exceed that observed in the reaction with the lighter isotope $^{239}\mathrm{Pu}$ by a factor of 10. The decay properties of the synthesized nuclei and their production cross sections indicate a rapid decrease of stability of superheavy nuclei as the neutron number decreases from the predicted magic neutron number $N=184$.

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