Beyond fossil fuel–driven nitrogen transformations
Jingguang G. ChenChemistry Division, Brookhaven National Laboratory, Upton, NY 11973, USARichard M. CrooksDepartment of Chemistry, The University of Texas at Austin, Austin, TX 78712, USALance C. SeefeldtDepartment of Chemistry and Biochemistry, Utah State University, Logan, UT 84332, USAKara L. BrenDepartment of Chemistry, University of Rochester, Rochester, NY 14627, USAR. Morris BullockPacific Northwest National Laboratory, Richland, WA 99352, USAMarcetta Y. DarensbourgDepartment of Chemistry, Texas A&M University, College Station, TX 77843, USAPatrick L. HollandDepartment of Chemistry, Yale University, New Haven, CT 06511, USABrian M. HoffmanDepartment of Chemistry, Northwestern University, Evanston, IL 60208, USAMichael J. JanikDepartment of Chemical Engineering, Pennsylvania State University, University Park, PA 16802, USAAnne K. JonesSchool of Molecular Sciences, Arizona State University, Tempe, AZ 85282, USAMercouri G. KanatzidisDepartment of Chemistry, Northwestern University, Evanston, IL 60208, USAPaul W. KingNational Renewable Energy Laboratory, Golden, CO 80401, USAKyle M. LancasterDepartment of Chemistry and Chemical Biology, Cornell University, Baker Laboratory, Ithaca, NY 14853, USASergei V. LymarChemistry Division, Brookhaven National Laboratory, Upton, NY 11973, USAPeter H. PfrommVoiland School of Chemical Engineering and Bioengineering, Washington State University, Pullman, WA 99164-6515, USAWilliam F. SchneiderDepartment of Chemical and Biomolecular Engineering, University of Notre Dame, Notre Dame, IN 46556, USARichard R. SchrockDepartment of Chemistry, MIT, 6-331, Cambridge, MA 02139, USA
2018en
ABI
Аннотация
Nitrogen is fundamental to all of life and many industrial processes. The interchange of nitrogen oxidation states in the industrial production of ammonia, nitric acid, and other commodity chemicals is largely powered by fossil fuels. A key goal of contemporary research in the field of nitrogen chemistry is to minimize the use of fossil fuels by developing more efficient heterogeneous, homogeneous, photo-, and electrocatalytic processes or by adapting the enzymatic processes underlying the natural nitrogen cycle. These approaches, as well as the challenges involved, are discussed in this Review.
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