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High-Order Harmonic Generation in Au Nanoparticle-Contained Plasmas

Mottamchetty VenkateshThe Guo Photonics Laboratory, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, ChinaR. A. GaneevDepartment of Physics, American University of Sharjah, 26666 Sharjah, UAEDmitry S. IvanovDepartment of Laser Photonics and optoelectronics, ITMO University, 197101 St. Petersburg, RussiaGanjaboy S. BoltaevDepartment of Physics, American University of Sharjah, 26666 Sharjah, UAEVyacheslav V. KimDepartment of Physics, American University of Sharjah, 26666 Sharjah, UAEJingguang LiangThe Guo Photonics Laboratory, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, ChinaA. A. SamokhvalovDepartment of Laser Photonics and optoelectronics, ITMO University, 197101 St. Petersburg, RussiaAndrei V. KabashinAix Marseille Univ, CNRS, LP3, Campus de Luminy, Case 917, 13288 Marseille, FranceS. M. KlimentovNational Research Nuclear University MEPhI (Moscow Engineering Physics Institute), 115409 Moscow, RussiaMartı́n E. GarciaInstitute of Physics and Center for Interdisciplinary Nanostructure Science and Technology (CINSaT), University of Kassel, 34125 Kassel, GermanyChunlei GuoThe Guo Photonics Laboratory, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, China
Nanomaterialsjournal2020en
ABI

Аннотация

Gold nanoparticles (NPs) have a wide range of applications in various fields. Here, we present high-order nonlinear optical studies of the plasmas produced from ablation of Au bulk targets and Au NP films deposited on paper and glass substrates. Experimentally, we analyze high-order harmonic generation (HHG) from gold NPs-containing plasmas. The HHG is produced by 35-fs pulses at 800 and 400 nm, while the plasmas are produced by femtosecond (35 fs, 800 nm), picosecond (200 ps, 800 nm), and nanosecond (5 ns, 1064 nm) pulses, respectively. High-order harmonics produced from ablated Au NPs on paper were 40 times stronger than the HHG from that ablated from the Au bulk targets. Through molecular dynamic simulations, we investigate the formation of gold NPs during laser ablation of a metal surface under different conditions.

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