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Graphitic carbon nitride supported single-atom catalysts for efficient oxygen evolution reaction

Xiyu LiCollaborative Innovation Center of Chemistry for Energy MaterialsPeng CuiCollaborative Innovation Center of Chemistry for Energy MaterialsWenhui ZhongGuiyangJun LiCollaborative Innovation Center of Chemistry for Energy MaterialsXijun WangCollaborative Innovation Center of Chemistry for Energy MaterialsZhaowu WangHenan University of Science and TechnologyJun JiangCollaborative Innovation Center of Chemistry for Energy Materials
2016en
ABI

Аннотация

Based on DFT calculations, we propose a TM@CN hybrid structure, in which the single-atom transition metal (TM = Pt, Pd, Co, Ni, Cu) is supported by graphitic carbon nitride (g-CN), as a promising high-performance OER catalyst. Our work reveals the importance of local TM coordination in catalysts for the OER, which would lead to a new class of low-cost, durable and efficient OER catalysts.

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