High Charge Carrier Mobilities and Lifetimes in Organolead Trihalide Perovskites
Christian WehrenfennigOxford University, Clarendon Laboratory Parks Road Oxford OX1 3PU UKGiles E. EperonOxford University, Clarendon Laboratory Parks Road Oxford OX1 3PU UKMichael B. JohnstonOxford University, Clarendon Laboratory Parks Road Oxford OX1 3PU UKHenry J. SnaithOxford University, Clarendon Laboratory Parks Road Oxford OX1 3PU UKLaura M. HerzOxford University, Clarendon Laboratory Parks Road Oxford OX1 3PU UK
2013en
ABI
Аннотация
Organolead trihalide perovskites are shown to exhibit the best of both worlds: charge-carrier mobilities around 10 cm2 V−1 s−1 and low bi-molecular charge-recombination constants. The ratio of the two is found to defy the Langevin limit of kinetic charge capture by over four orders of magnitude. This mechanism causes long (micrometer) charge-pair diffusion lengths crucial for flat-heterojunction photovoltaics.
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