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Very large gold and silver sputtering yields induced by keV to MeV energy<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">Au</mml:mi></mml:mrow><mml:mrow><mml:mi>n</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math>clusters<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mo>(</mml:mo><mml:mi>n</mml:mi><mml:mo>=</mml:mo><mml:mn>1</mml:mn><mml:mn/><mml:mo>–</mml:mo><mml:mn>1</mml:mn><mml:mn>3</mml:mn><mml:mo>)</mml:mo></mml:math>

S. BouneauInstitut de Physique Nucléaire d’Orsay, UMR 8608, CNRS-IN2P3-Université Paris-Sud, 91406 Orsay Cedex, FranceAlain BrunelleInstitut de Physique Nucléaire d’Orsay, UMR 8608, CNRS-IN2P3-Université Paris-Sud, 91406 Orsay Cedex, FranceS. Della‐NegraInstitut de Physique Nucléaire d’Orsay, UMR 8608, CNRS-IN2P3-Université Paris-Sud, 91406 Orsay Cedex, FranceJ. DepauwInstitut National de Physique Nucléaire et de Physique des ParticulesD. JacquetInstitut de Physique Nucléaire d’Orsay, UMR 8608, CNRS-IN2P3-Université Paris-Sud, 91406 Orsay Cedex, FranceY. Le BeyecInstitut de Physique Nucléaire d’Orsay, UMR 8608, CNRS-IN2P3-Université Paris-Sud, 91406 Orsay Cedex, FranceM. PautratInstitut de Physique Nucléaire d’Orsay, UMR 8608, CNRS-IN2P3-Université Paris-Sud, 91406 Orsay Cedex, FranceM. FallavierInstitut de Physique Nucléaire de Lyon, UMR 5822, CNRS-IN2P3-Université Claude Bernard, 43 Boulevard du 11 novembre 1918, 69622 Villeurbanne Cedex, FranceJean-Claude PoizatInstitut de Physique Nucléaire de Lyon, UMR 5822, CNRS-IN2P3-Université Claude Bernard, 43 Boulevard du 11 novembre 1918, 69622 Villeurbanne Cedex, FranceHans Henrik AndersenNiels Bohr Institute, Ørsted Laboratory, Universitetsparken 5, DK-2100 Copenhagen Ø, Denmark
2002lv
ABI

Аннотация

The total sputtering yields of gold and silver targets bombarded by ${\mathrm{Au}}_{n}$ $(n=1--13)$ clusters have been measured over a broad range of incident energy per atom (from 20 keV/atom to 5 MeV/atom). Large nonlinear effects in the sputtering yields were observed. For silver targets, yield values as high as \ensuremath{\sim}20 000 atoms per impact of ${\mathrm{Au}}_{13}$ at 1.2 MeV (92 keV/atom) were measured while only 45 atoms are emitted from the same target in the impact of single gold atoms at the same energy per atom. The sputtering yield variation with incident projectile energy per atom shows that maxima occur at \ensuremath{\sim}250 keV/atom for a gold target and \ensuremath{\sim}150 keV/atom for a silver target for projectiles with three or more atoms. In both cases the maxima of nuclear stopping power are at much larger energies per atom (700 keV for Au on Au and 550 keV for Au on Ag). Large surface deformations with craters and rims are observed by atomic force microscopy at the surface of cluster irradiated targets. Their number per unit area corresponds to the irradiation fluence and they are of approximately the same size, demonstrating that fluctuations between events are small.

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