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Crystal growth and optical characterization of cerium-doped Lu1.8Y0.2SiO5

D. W. CookeMaterials Science and Technology Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545Kenneth J. McClellanMaterials Science and Technology Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545Bryan BennettMaterials Science and Technology Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545J. M. RoperMaterials Science and Technology Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545Mark WhittakerMaterials Science and Technology Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545R. E. MuenchausenMaterials Science and Technology Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545Robert C. SzeChemical Sciences and Technology Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545
2000en
ABI

Аннотация

Czochralski growth of cerium-doped Lu1.8Y0.2SiO5 (LYSO) from a 90/10 solution of Lu2SiO5 (LSO) and Y2SiO5 (YSO) is demonstrated. The alloyed scintillator retains the favorable growth properties of YSO and the desirable physical and optical scintillator properties of LSO. Radioluminescence, thermally stimulated luminescence, optical absorption, and lifetime measurements confirm the equivalence of LYSO and LSO optical properties. Advantages of LYSO Czochralski growth relative to LSO include reduced melting point, less propensity for formation of crystalline inclusions, lower cost of starting material, and easier incorporation of cerium into the host lattice. This material offers an attractive alternative to LSO for scintillator applications.

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