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Nonlinear Optical Characterization of 2D Materials

Linlin ZhouWuhan National Laboratory for Optoelectronics, School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan 430074, ChinaHuange FuWuhan National Laboratory for Optoelectronics, School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan 430074, ChinaTing LvWuhan National Laboratory for Optoelectronics, School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan 430074, ChinaChengbo WangWuhan National Laboratory for Optoelectronics, School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan 430074, ChinaHui GaoWuhan National Laboratory for Optoelectronics, School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan 430074, ChinaDaqian LiWuhan National Laboratory for Optoelectronics, School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan 430074, ChinaLeimin DengWuhan National Laboratory for Optoelectronics, School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan 430074, ChinaWei XiongWuhan National Laboratory for Optoelectronics, School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan 430074, China
2020en
ABI

Аннотация

Characterizing the physical and chemical properties of two-dimensional (2D) materials is of great significance for performance analysis and functional device applications. As a powerful characterization method, nonlinear optics (NLO) spectroscopy has been widely used in the characterization of 2D materials. Here, we summarize the research progress of NLO in 2D materials characterization. First, we introduce the principles of NLO and common detection methods. Second, we introduce the recent research progress on the NLO characterization of several important properties of 2D materials, including the number of layers, crystal orientation, crystal phase, defects, chemical specificity, strain, chemical dynamics, and ultrafast dynamics of excitons and phonons, aiming to provide a comprehensive review on laser-based characterization for exploring 2D material properties. Finally, the future development trends, challenges of advanced equipment construction, and issues of signal modulation are discussed. In particular, we also discuss the machine learning and stimulated Raman scattering (SRS) technologies which are expected to provide promising opportunities for 2D material characterization.

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