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Highly Efficient and Stable White Light‐Emitting Diodes Using Perovskite Quantum Dot Paper

Chieh‐Yu KangDepartment of Photonics and Institute of Electro‐Optical Engineering College of Electrical and Computer Engineering National Chiao Tung University Hsinchu 30010 Taiwan Republic of ChinaChun‐Ho LinComputer, Electrical, and Mathematical Sciences and Engineering Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955‐6900 Saudi ArabiaChih‐Hao LinComputer, Electrical, and Mathematical Sciences and Engineering Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955‐6900 Saudi ArabiaTing LiComputer, Electrical, and Mathematical Sciences and Engineering Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955‐6900 Saudi ArabiaSung‐Wen Huang ChenDepartment of Photonics and Institute of Electro‐Optical Engineering College of Electrical and Computer Engineering National Chiao Tung University Hsinchu 30010 Taiwan Republic of ChinaChun‐Lin TsaiDepartment of Photonics and Institute of Electro‐Optical Engineering College of Electrical and Computer Engineering National Chiao Tung University Hsinchu 30010 Taiwan Republic of ChinaChin‐Wei SherDepartment of Photonics and Institute of Electro‐Optical Engineering College of Electrical and Computer Engineering National Chiao Tung University Hsinchu 30010 Taiwan Republic of ChinaTingzhu WuDepartment of Photonics and Institute of Electro‐Optical Engineering College of Electrical and Computer Engineering National Chiao Tung University Hsinchu 30010 Taiwan Republic of ChinaPo‐Tsung LeeDepartment of Photonics and Institute of Electro‐Optical Engineering College of Electrical and Computer Engineering National Chiao Tung University Hsinchu 30010 Taiwan Republic of ChinaXuezhu XuComputer, Electrical, and Mathematical Sciences and Engineering Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955‐6900 Saudi ArabiaMaolin ZhangComputer, Electrical, and Mathematical Sciences and Engineering Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955‐6900 Saudi ArabiaChih‐Hsiang HoJr‐Hau HeComputer, Electrical, and Mathematical Sciences and Engineering Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955‐6900 Saudi ArabiaHao‐Chung KuoDepartment of Photonics and Institute of Electro‐Optical Engineering College of Electrical and Computer Engineering National Chiao Tung University Hsinchu 30010 Taiwan Republic of China
2019en
ABI

Аннотация

Abstract Perovskite quantum dots (PQDs) are a competitive candidate for next‐generation display technologies as a result of their superior photoluminescence, narrow emission, high quantum yield, and color tunability. However, due to poor thermal resistance and instability under high energy radiation, most PQD‐based white light‐emitting diodes (LEDs) show only modest luminous efficiency of ≈50 lm W −1 and a short lifetime of <100 h. In this study, by incorporating cellulose nanocrystals, a new type of QD film is fabricated: CH 3 NH 3 PbBr 3 PQD paper that features 91% optical absorption, intense green light emission (518 nm), and excellent stability attributed to the complexation effect between the nanocellulose and PQDs. The PQD paper is combined with red K 2 SiF 6 :Mn4 + phosphor and blue GaN LED chips to fabricate a high‐performance white LED demonstrating ultrahigh luminous efficiency (124 lm W −1 ), wide color gamut (123% of National Television System Committee), and long operation lifetime (240 h), which paves the way for advanced lighting technology.

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