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Design of N-Coordinated Dual-Metal Sites: A Stable and Active Pt-Free Catalyst for Acidic Oxygen Reduction Reaction

Jing WangDepartment of Chemistry, iChEM (Collaborative Innovation Center of Chemistry for Energy Materials), University of Science and Technology of China, Hefei 230026, ChinaZheng‐Qing HuangInstitute of Industrial Catalysis, School of Chemical Engineering and Technology, Xi’an Jiaotong University, Xi’an 710049, ChinaWei LiuHefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei 230026, ChinaChun‐Ran ChangInstitute of Industrial Catalysis, School of Chemical Engineering and Technology, Xi’an Jiaotong University, Xi’an 710049, ChinaHaolin TangState Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, ChinaZhijun LiDepartment of Chemistry, Queen’s University, Kingston, Ontario K7L 3N6, CanadaWenxing ChenDepartment of Chemistry, Tsinghua University, Beijing 100084, ChinaChun‐Jiang JiaKey Laboratory for Colloid and Interface Chemistry, Key Laboratory of Special Aggregated Materials, School of Chemistry and Chemical Engineering, Shandong University, Jinan 250100, ChinaTao YaoHefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei 230026, ChinaShiqiang WeiHefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei 230026, ChinaYuen WuDepartment of Chemistry, iChEM (Collaborative Innovation Center of Chemistry for Energy Materials), University of Science and Technology of China, Hefei 230026, ChinaYadong LiDepartment of Chemistry, Tsinghua University, Beijing 100084, China
2017en
ABI

Аннотация

/air single cell operation. Density functional theory calculations reveal the dual sites is favored for activation of O-O, crucial for four-electron oxygen reduction.

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