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A wide-frequency range dielectric tuning of BaTiO<sub>3</sub>by embedding metal nanocrystals

Zhengwei XiongJoint Laboratory for Extreme Conditions Matter PropertiesQian LiuMianyangJinlong TangChinaLeiming FangMianyangXiaoqiang ZhangChina Academy of Engineering PhysicsJun LiChina Academy of Engineering PhysicsYajun FuChinaJin WangMianyangZhipeng GaoInstitute of Fluid PhysicsDeli ShiJoint Laboratory for Extreme Conditions Matter Properties
RSC Advancesjournal2021en
ABI

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(BTO) matrix. According to optimized growth processes, a novel nanocomposite system was constructed, which consisted a well epitaxial BTO layer and three-dimensional Fe NCs. Based on this, the different dielectric response in the regions of low temperature-high frequency and low frequency-high temperature were revealed by the contribution of hopping and interfacial polarizations, respectively. With the increased amount of Fe NCs, the obvious enhancement in the low-frequency conductivity, middle frequency capacitance, and high-frequency inductive effect was found. The embedded metal NCs play an important role in tuning the dielectric behaviors and AC conductivity of oxide dielectrics. This significant rectification effect in wide-frequency ranges opens up a new direction for designing embedded nano-capacitors.

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