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Probing the spin dynamics of quasi-2D magnets Cu(1,3-bdc) using a superconducting resonator

Chenyu LiSchool of Microelectronics, University of Science and Technology of China 1 , Hefei,Yujia FanSchool of Microelectronics, University of Science and Technology of China 1 , Hefei,Wenjie DingSchool of Microelectronics, University of Science and Technology of China 1 , Hefei,Kang WangAnhui Province Key Laboratory of Low-Energy Quantum Materials and Devices, High Magnetic Field Laboratory, HFIPS, Chinese Academy of Sciences 2 , Hefei, Anhui 230031,Chao ZhouHefei Institutes of Physical Science, Chinese Academy of Science 3 , Hefei 230031,Dongsheng SongInformation Materials and Intelligent Sensing Laboratory of Anhui Province, Anhui Key Laboratory of Magnetic Functional Materials and Devices, Institutes of Physical Science and Information Technology, Anhui University 4 , Hefei,Lichuan ZhangFaculty of Physics and Electronic Engineering, Jiangsu University 5 , Zhenjiang 212013,Yuriy MokrousovPeter Grünberg Institut and Institute for Advanced Simulation, Forschungszentrum Jülich and JARA 6 , 52425 Jülich,Shiming LeiHong Kong University of Science and Technology 8 , Clear Water Bay,P. B. ParchinskiyDepartment of Semiconductor and Polymer Physics, National University of Uzbekistan 9 , Tashkent 100174,Haifeng DuHigh Magnetic Field LaboratoryLihui BaiState Key Laboratory of Crystal MaterialsPeng GaoHefei Institutes of Physical Science, Chinese Academy of Science 3 , Hefei 230031,Tao YuSchool of Physics, Huazhong University of Science and Technology 11 , Wuhan 430074,Yi‐Pu WangZhejiang Key Laboratory of Micro-Nano Quantum Chips and Quantum Control, School of Physics, and State Key Laboratory for Extreme Photonics and Instrumentation, Zhejiang University 12 , Hangzhou 310027,Tianxiang NanSchool of Integrated Circuits and Beijing National Research Center for Information Science and Technology (BNRist), Tsinghua University 13 , Beijing,Peng LiSchool of Microelectronics, University of Science and Technology of China 1 , Hefei,
Applied Physics Lettersjournal2025en

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Quantum magnonics presents significant potential for advancing quantum sensors through magnon–photon coupling. In this research, we experimentally and theoretically study the microwave-mediated coherent coupling in a system combined by a superconducting resonator chip and quasi-two-dimensional topological magnets Cu[1,3-benzenedicarboxylate(bdc)]. By changing the orientation of the Cu(1,3-bdc) flakes on the chip, coherent level repulsion of two different magnon modes is demonstrated. Our measurements indicate that magnon modes in two anisotropic Cu(1,3-bdc) flakes interact with each other by the mediation of cavity photons, with the coupling energy transfer conforming to the “magnon-loss-resistor” model. Our research offers a pathway to investigate spin dynamics in innovative quantum materials, facilitating magnon–photon coupling for effective quantum operations.

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