A scalable metal-organic framework as a durable physisorbent for carbon dioxide capture
Jian‐Bin LinDepartment of Chemistry, University of Calgary, Calgary, Alberta, CanadaTai NguyenDepartment of Chemical and Materials Engineering, University of Alberta, Edmonton, Alberta, CanadaRamanathan VaidhyanathanIndian Institute of Science Education and Research, Dr. Homi Bhabha Road, Pashan, Pune, Maharashtra, 411008, IndiaJake BurnerDepartment of Chemistry and Biomolecular Science, University of Ottawa, Ottawa, Ontario, CanadaJared M. TaylorZoraMat Solutions Inc., Calgary, Alberta, CanadaHana DurekovaDepartment of Chemistry and Biomolecular Science, University of Ottawa, Ottawa, Ontario, CanadaFarid AkhtarDepartment of Materials Engineering, Luleå University of Technology, Luleå, SwedenRoger K. MahDepartment of Chemistry, University of Calgary, Calgary, Alberta, CanadaOmid Ghaffari NikSvante Inc., Vancouver, British Columbia, CanadaStefan MarxBASF SE, Ludwigshafen am Rhein, GermanyNicholas FylstraDepartment of Chemistry, University of Calgary, Calgary, Alberta, CanadaS.S. IremongerDepartment of Chemistry, University of Calgary, Calgary, Alberta, CanadaKarl W. DawsonDepartment of Chemistry, University of Calgary, Calgary, Alberta, CanadaPartha SarkarDepartment of Chemical and Materials Engineering, University of Alberta, Edmonton, Alberta, CanadaPierre HovingtonSvante Inc., Vancouver, British Columbia, CanadaArvind RajendranDepartment of Chemical and Materials Engineering, University of Alberta, Edmonton, Alberta, CanadaTom K. WooDepartment of Chemistry and Biomolecular Science, University of Ottawa, Ottawa, Ontario, CanadaGeorge K. H. ShimizuZoraMat Solutions Inc., Calgary, Alberta, Canada
2021en
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ABI
Annotatsiya
A hydrophobic CO 2 physisorbent Most materials for carbon dioxide (CO 2 ) capture of fossil fuel combustion, such as amines, rely on strong chemisorption interactions that are highly selective but can incur a large energy penalty to release CO 2 . Lin et al . show that a zinc-based metal organic framework material can physisorb CO 2 and incurs a lower regeneration penalty. Its binding site at the center of the pores precludes the formation of hydrogen-bonding networks between water molecules. This durable material can preferentially adsorb CO2 at 40% relative humidity and maintains its performance under flue gas conditions of 150°C. —PDS
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