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Estimation of 99Mo production rates from natural molybdenum in research reactors

M. BlaauwReactor Institute Delft, Delft University of Technology, Mekelweg 15, 2629 JB Delft, The NetherlandsD. RidikasDivision of Physical and Chemical Sciences, Department of Nuclear Sciences and Applications, International Atomic Energy Agency, Vienna, AustriaS.A. BaytelesovInstitute of Nuclear Physics, Academy of Sciences of Uzbekistan, Ulug Gulomov Str., Tashkent, Uzbekistan 100214Pep SalasInstituto Peruano de Energia Nuclear, Avenida Canadá 1470, 41, Lima, PeruY. ChakrovaInstitute of Nuclear Physics of Ministry of Energy of the Republic of Kazakhstan, Ibragimova 1, Almaty, Kazakhstan 050032Eun-Ha ChoRI Research Division, Korea Atomic Energy Research Institute, 989-111, Daedeok-daero, Yuseong-gu, Daejeon 305-353 KoreaRehir DahalanMedical Technology Division, Malaysian Nuclear Agency, Bangi, 43000 Kajang, Selangor MalaysiaA. H. FortunatoInstituto Nacionale de Investigciones Nucleares, Carretera Mexico-Toluca S/N La Marquesa, Ocoyoacac, MexicoRadojko JačimovićJozef Stefan Institute, Jamova Cesta 39, 1000 Ljubljana, SloveniaA. KlingCentro de Ciências e Tecnologias Nucleares and Laboratório de Engenharia Nuclear, Instituto Superior Técnico, Universidade de Lisboa, E.N. 10 ao km 139,7,, 2695-066 Bobadela LRS, PortugalLorena MuñozComisión Chilena de Energía Nuclear (CCHEN), Avenida Nueva Bilbao No. 12501, Las Condes, Santiago, ChileNader M. A. MohamedEgypt Second Research Reactor (ETRR-2), Atomic Energy Authority (AEA), Abou Zabal, Cairo, 13759 EgyptDénes PárkányiCentre for Energy Research, Hungarian Academy of Sciences, Konkoly Thege Miklós út 29-33, Budapest, 1121 HungaryTej Pratap SinghDepartment of Atomic Energy (DAE), Bhabha Atomic Research Centre (BARC), Trombay, Mumbai, Maharashtra 400 085 IndiaVan Dong DuongVietnam Atomic Energy Institute, 01 Nguyen Tu Luc, Dalat, Vietnam
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Annotatsiya

Molybdenum-99 is one of the most important radionuclides for medical diagnostics. In 2015, the International Atomic Energy Agency organized a round-robin exercise where the participants measured and calculated specific saturation activities achievable for the 98Mo(n,γ)99Mo reaction. This reaction is of interest as a means to locally, and on a small scale, produce 99Mo from natural molybdenum. The current paper summarises a set of experimental results and reviews the methodology for calculating the corresponding saturation activities. Activation by epithermal neutrons and also epithermal neutron self-shielding are found to be of high importance in this case.

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