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Relationship between Particle Mass and Mobility for Diesel Exhaust Particles

Kihong ParkDepartment of Mechanical Engineering, University of Minnesota, 111 Church Street SE, Minneapolis, Minnesota 55455Feng CaoDepartment of Mechanical Engineering, University of Minnesota, 111 Church Street SE, Minneapolis, Minnesota 55455David B. KittelsonDepartment of Mechanical Engineering, University of Minnesota, 111 Church Street SE, Minneapolis, Minnesota 55455Peter H. McMurryDepartment of Mechanical Engineering, University of Minnesota, 111 Church Street SE, Minneapolis, Minnesota 55455

2002en

ABI

Annotatsiya

We used the aerosol particle mass analyzer (APM) to measure the mass of mobility-classified diesel exhaust particles. This information enabled us to determine the effective density and fractal dimension of diesel particles as a function of engine load. We found that the effective density decreases as particle size increases. TEM images showed that this occurs because particles become more highly agglomerated as size increases. Effective density and fractal dimension increased somewhat as engine load decreased. TEM images suggest that this occurs because these particles contain more condensed fuel and/or lubricating oil. Also, we observed higher effective densities when high-sulfur EPA fuel (approximately 360 ppm S) was used than for Fischer-Tropsch fuel (approximately 0 ppm S). In addition, the effective density provides the relationship between mobility and aerodynamic equivalent diameters. The relationship between these diameters enables us to intercompare, in terms of a common measure of size, mass distributions measured with the scanning mobility particle sizer (SMPS) and a MOUDI impactor without making any assumptions about particle shape or density. We show that mass distributions of diesel particles measured with the SMPS-APM are in good agreement with distributions measured with a MOUDI and a nano-MOUDI for particles larger than approximately 60 nm. However, significantly more mass and greater variation were observed by the nano-MOUDI for particles smaller than 40 nm than by the SMPS-APM.

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Identifikatorlar

DOI: 10.1021/es025960v

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