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Emerging Device Applications for Semiconducting Two-Dimensional Transition Metal Dichalcogenides

Deep JariwalaDepartment of Materials Science and Engineering, ‡Department of Chemistry, and §Department of Medicine, Northwestern University, Evanston, Illinois 60208, United StatesVinod K. SangwanDepartment of Materials Science and Engineering, ‡Department of Chemistry, and §Department of Medicine, Northwestern University, Evanston, Illinois 60208, United StatesLincoln J. LauhonDepartment of Materials Science and Engineering, ‡Department of Chemistry, and §Department of Medicine, Northwestern University, Evanston, Illinois 60208, United StatesTobin J. MarksDepartment of Materials Science and Engineering, ‡Department of Chemistry, and §Department of Medicine, Northwestern University, Evanston, Illinois 60208, United StatesMark C. HersamDepartment of Materials Science and Engineering, ‡Department of Chemistry, and §Department of Medicine, Northwestern University, Evanston, Illinois 60208, United States
2014en
ABI

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With advances in exfoliation and synthetic techniques, atomically thin films of semiconducting transition metal dichalcogenides have recently been isolated and characterized. Their two-dimensional structure, coupled with a direct band gap in the visible portion of the electromagnetic spectrum, suggests suitability for digital electronics and optoelectronics. Toward that end, several classes of high-performance devices have been reported along with significant progress in understanding their physical properties. Here, we present a review of the architecture, operating principles, and physics of electronic and optoelectronic devices based on ultrathin transition metal dichalcogenide semiconductors. By critically assessing and comparing the performance of these devices with competing technologies, the merits and shortcomings of this emerging class of electronic materials are identified, thereby providing a roadmap for future development.

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