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Observation of resonance-enhanced high-order harmonics from direct excitation of metal nanoparticles with femtosecond pulses

Jingguang LiangGPL, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, ChinaYu Hang LaiGPL, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, ChinaWufeng FuGPL, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, ChinaYuwei ShanGPL, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, ChinaWeili YuGPL, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, ChinaChunlei GuoThe Institute of Optics, University of Rochester, Rochester, New York 14627, USA
2020en
ABI

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We report on the observation of resonance enhanced high-order harmonic generation (HHG) from a dense medium composed of indium or tin nanoparticles. Unlike previous studies of resonance enhanced high harmonics from laser produced plasma plume from a prepulse, we generate HHG directly, thus eliminating the undesired contributions from various components in the plasma. We discuss the mechanisms for our observed resonance effect in the absence of preionized particles and the implications of the experimental results on the HHG mechanism in metal nanoparticles.

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