Capture of CO<sub>2</sub> from N<sub>2</sub> and CH<sub>4</sub> over a wide temperature range on a robust MOF with Brønsted acidic and Lewis basic dual functional sites
Shijian LuJiangsu Key Laboratory of Coal-based Greenhouse Gas Control and Utilization, Carbon Neutrality Institute, China University of Mining and Technology, Xuzhou, 221116, P. R. ChinaYajie ZhangSchool of Materials and Physics, China University of Mining and Technology, Xuzhou 221116, P. R. ChinaYi-Ting ChengSchool of Materials and Physics, China University of Mining and Technology, Xuzhou 221116, P. R. ChinaZi-Heng QinSchool of Materials and Physics, China University of Mining and Technology, Xuzhou 221116, P. R. ChinaGang‐Ding WangKey Laboratory of Synthetic and Natural Functional Molecule of the Ministry of Education, Shaanxi Key Laboratory of Physico-Inorganic Chemistry, College of Chemistry & Materials Science, Northwest University, Xi'an 710069, P. R. ChinaYuan BaiGuodian Environmental Research Institute Co., Ltd., Nanjing 210031, ChinaYichao LinSchool of Safety Engineering, China University of Mining and Technology, Xuzhou 221116, Jiangsu, ChinaHetang WangSchool of Safety Engineering, China University of Mining and Technology, Xuzhou 221116, Jiangsu, ChinaYanwei SuiSchool of Materials and Physics, China University of Mining and Technology, Xuzhou 221116, P. R. ChinaLei HouKey Laboratory of Synthetic and Natural Functional Molecule of the Ministry of Education, Shaanxi Key Laboratory of Physico-Inorganic Chemistry, College of Chemistry & Materials Science, Northwest University, Xi'an 710069, P. R. ChinaYong-Zhi LiSchool of Materials and Physics, China University of Mining and Technology, Xuzhou 221116, P. R. China
2025en
ABI
Annotatsiya
A robust MOF (CUMT-1a) with Lewis basic and Brønsted acidic dual functional sites is designed and constructed, which can simultaneously afford high-purity N 2 , CH 4 and CO 2 from CO 2 /N 2 , CO 2 /CH 4 and CO 2 /CH 4 /N 2 mixtures over a wide temperature range.
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