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Preventing Graphene Sheets from Restacking for High-Capacitance Performance

Yan WangKey Laboratory of Functional Polymer Materials and Center for Nanoscale Science and Technology, Institute of Polymer Chemistry, College of Chemistry, Nankai University, Weijin Road 94, Tianjin 300071, ChinaYingpeng WuKey Laboratory of Functional Polymer Materials and Center for Nanoscale Science and Technology, Institute of Polymer Chemistry, College of Chemistry, Nankai University, Weijin Road 94, Tianjin 300071, ChinaYi HuangKey Laboratory of Functional Polymer Materials and Center for Nanoscale Science and Technology, Institute of Polymer Chemistry, College of Chemistry, Nankai University, Weijin Road 94, Tianjin 300071, ChinaFan ZhangKey Laboratory of Functional Polymer Materials and Center for Nanoscale Science and Technology, Institute of Polymer Chemistry, College of Chemistry, Nankai University, Weijin Road 94, Tianjin 300071, ChinaXi YangKey Laboratory of Functional Polymer Materials and Center for Nanoscale Science and Technology, Institute of Polymer Chemistry, College of Chemistry, Nankai University, Weijin Road 94, Tianjin 300071, ChinaYanfeng MaKey Laboratory of Functional Polymer Materials and Center for Nanoscale Science and Technology, Institute of Polymer Chemistry, College of Chemistry, Nankai University, Weijin Road 94, Tianjin 300071, ChinaYongsheng ChenKey Laboratory of Functional Polymer Materials and Center for Nanoscale Science and Technology, Institute of Polymer Chemistry, College of Chemistry, Nankai University, Weijin Road 94, Tianjin 300071, China
2011en
ABI

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Aiming at preventing restacking of individual graphene sheets by using a simple green hydrothermal route, we have introduced carbon nanotubes to act as the spacer in fabricating a three-dimensional (3-D) hierarchical structure with graphene sheets. These 3-D hierarchical structure materials have been used to fabricate supercapacitor devices, and a high specific capacitance of 318 F/g for graphene with an energy density of 11.1 (W h)/kg has been achieved.

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