Tracking the photodissociation probability of D2+ induced by linearly chirped laser pulses
András CsehiUniversity of Debrecen 1 Department of Theoretical Physics, , P.O. Box 5, H-4010 Debrecen, HungaryGábor J. HalászUniversity of Debrecen 2 Department of Information Technology, , P.O. Box 12, H-4010 Debrecen, HungaryLorenz S. CederbaumUniversität Heidelberg 3 Theoretische Chemie, Physikalish-Chemisches Institut, , H-69120 Heidelberg, GermanyÁgnes VibókELI-HU Non-Profit Ltd 4 ELI-ALPS, , Dugonics tér 13, H-6720 Szeged, Hungary
2016en
ABI
Annotatsiya
In the presence of linearly varying frequency chirped laser pulses, the photodissociation dynamics of D2(+) is studied theoretically after ionization of D2. As a completion of our recent work [A. Csehi et al., J. Chem. Phys. 143, 014305 (2015)], a comprehensive dependence on the pulse duration and delay time is presented in terms of total dissociation probabilities. Our numerical analysis carried out in the recently introduced light-induced conical intersection (LICI) framework clearly shows the effects of the changing position of the LICI which is induced by the frequency modulation of the chirped laser pulses. This impact is presented for positively, negatively, and zero chirped short pulses.
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