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Roadmap on organic–inorganic hybrid perovskite semiconductors and devices

Lukas Schmidt‐MendeDepartment of Physics, University of Konstanz 1 , Universitaetsstr. 10, 78457 Konstanz, GermanyVladimir DyakonovExperimental Physics VI, University of Würzburg 2 , Am Hubland, 97074 Würzburg, GermanySelina OlthofDepartment of Chemistry, University of Cologne 3 , Greinstraße 4-6, 50939 Cologne, GermanyFeray ÜnlüDepartment of Chemistry, University of Cologne 3 , Greinstraße 4-6, 50939 Cologne, GermanyKhan LêDepartment of Chemistry, University of Cologne 3 , Greinstraße 4-6, 50939 Cologne, GermanySanjay MathurDepartment of Chemistry, University of Cologne 3 , Greinstraße 4-6, 50939 Cologne, GermanyAndrei KarabanovInstitute for Materials Science and Center for Nanointegration Duisburg-Essen (CENIDE), University of Duisburg-Essen 4 , 45141 Essen, GermanyDoru C. LupascuInstitute for Materials Science and Center for Nanointegration Duisburg-Essen (CENIDE), University of Duisburg-Essen 4 , 45141 Essen, GermanyLaura M. HerzClarendon Laboratory, Department of Physics, University of Oxford 5 , Parks Road, Oxford OX1 3PU, United KingdomAlexander HinderhoferInstitute of Applied Physics, University of Tübingen 7 , Auf der Morgenstelle 10, 72076 Tübingen, GermanyFrank SchreiberInstitute of Applied Physics, University of Tübingen 7 , Auf der Morgenstelle 10, 72076 Tübingen, GermanyAlexey ChernikovDepartment of Physics, University of Regensburg 8 , 93053 Regensburg, GermanyDavid A. EggerDepartment of Physics, Technical University of Munich 10 , 85748 Garching, GermanyOleksandra ShargaievaHelmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group ‘Hybrid Materials Formation and Scaling 11 ,’ Kekulestr. 5, 12489 Berlin, GermanyCaterina CocchiHelmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group ‘Hybrid Materials Formation and Scaling 11 ,’ Kekulestr. 5, 12489 Berlin, GermanyEva UngerHelmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group ‘Hybrid Materials Formation and Scaling 11 ,’ Kekulestr. 5, 12489 Berlin, GermanyMichael SalibaCarl von Ossietzky Universität Oldenburg, Institute of Physics 12 , Carl-von-Ossietzky-Straße 9, 26129 Oldenburg, GermanyMahdi Malekshahi ByranvandHelmholtz Young Investigator Group, lEK5-Photovoltaik, Forschungszentrum Jülich 13 , Pfaffenwaldring 47, 70569 Stuttgart, Germany and , 52425 Jülich, GermanyMartin KrollDresden Integrated Center for Applied Physics and Photonic Materials (IAPP), Technische Universität Dresden 14 , 01062 Dresden, GermanyFrederik NehmDepartment of Physics and Materials Science, University of Luxembourg 15 , Luxembourg, LuxembourgKarl LeoDresden Integrated Center for Applied Physics and Photonic Materials (IAPP), Technische Universität Dresden 14 , 01062 Dresden, GermanyAlex RedingerDepartment of Physics and Materials Science, University of Luxembourg 15 , Luxembourg, LuxembourgJulian HöckerExperimental Physics VI, University of Würzburg 2 , Am Hubland, 97074 Würzburg, GermanyThomas KirchartzFaculty of Engineering and CENIDE, University of Duisburg-Essen 16 , 52425 Jülich, Germany and , Carl-Benz-Str. 199, 47057 Duisburg, GermanyJonathan WarbyInstitute of Physics and Astronomy, University of Potsdam 17 , Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, GermanyEmilio Gutierrez‐PartidaInstitute of Physics and Astronomy, University of Potsdam 17 , Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, GermanyDieter NeherInstitute of Physics and Astronomy, University of Potsdam 17 , Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, GermanyMartin StolterfohtInstitute of Physics and Astronomy, University of Potsdam 17 , Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, GermanyUli WürfelDepartment of Organic and Perovskite Photovoltaics, Fraunhofer Institute for Solar Energy Systems (ISE) 19 , Heidenhofstraße 2, 79110 Freiburg, GermanyMoritz UnmüssigDepartment of Organic and Perovskite Photovoltaics, Fraunhofer Institute for Solar Energy Systems (ISE) 19 , Heidenhofstraße 2, 79110 Freiburg, GermanyJan HerterichDepartment of Organic and Perovskite Photovoltaics, Fraunhofer Institute for Solar Energy Systems (ISE) 19 , Heidenhofstraße 2, 79110 Freiburg, GermanyClemens BaretzkyDepartment of Organic and Perovskite Photovoltaics, Fraunhofer Institute for Solar Energy Systems (ISE) 19 , Heidenhofstraße 2, 79110 Freiburg, GermanyJohn MohanrajApplied Functional Polymers, Macromolecular Chemistry I, University of Bayreuth 20 , 95440 Bayreuth, GermanyMukundan ThelakkatApplied Functional Polymers, Macromolecular Chemistry I, University of Bayreuth 20 , 95440 Bayreuth, GermanyClément MaheuSurface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt 22 , Otto-Berndt-Strasse 3, 64287 Darmstadt, GermanyWolfram JaegermannSurface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt 22 , Otto-Berndt-Strasse 3, 64287 Darmstadt, GermanyThomas MayerSurface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt 22 , Otto-Berndt-Strasse 3, 64287 Darmstadt, GermanyJanek RiegerLehrstuhl für Festkörperphysik, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU) 23 , Staudtstr. 7, 91058 Erlangen, GermanyThomas FausterLehrstuhl für Festkörperphysik, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU) 23 , Staudtstr. 7, 91058 Erlangen, GermanyDaniel NiesnerLehrstuhl für Festkörperphysik, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU) 23 , Staudtstr. 7, 91058 Erlangen, GermanyFengjiu YangHelmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group Perovskite Tandem Solar Cells 24 , 12489 Berlin, GermanySteve AlbrechtHelmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group Perovskite Tandem Solar Cells 24 , 12489 Berlin, GermanyThomas RiedlInstitute of Electronic Devices, University of Wuppertal 26 , 42119 Wuppertal, GermanyAzhar FakharuddinDepartment of Physics, University of Konstanz 1 , Universitaetsstr. 10, 78457 Konstanz, GermanyMaria VasilopoulouInstitute of Nanoscience and Nanotechnology, National Center for Scientific Research Demokritos 28 , 15341 Agia Paraskevi, Attica, GreeceYana VaynzofIntegrated Center for Applied Physics and Photonic Materials (IAPP) and Center for Advancing Electronics Dresden (cfaed), Technische Universität Dresden 29 , Nöthnitzer Straße 61, 01187 Dresden, GermanyDavide MoiaMax Planck Institute for Solid State Research 30 , Heisenbergstrasse 1, 70569 Stuttgart, GermanyJoachim MaierMax Planck Institute for Solid State Research 30 , Heisenbergstrasse 1, 70569 Stuttgart, GermanyMarius FranckevičiusDepartment of Molecular Compound Physics, Center for Physical Sciences and Technology 31 (FTMC), Saulėtekio Avenue 3, Vilnius LT-10257, LithuaniaVidmantas GulbinasDepartment of Molecular Compound Physics, Center for Physical Sciences and Technology 31 (FTMC), Saulėtekio Avenue 3, Vilnius LT-10257, LithuaniaRoss A. KernerDepartment of Electrical Engineering, Princeton University 32 , Princeton, New Jersey 08544, USALianfeng ZhaoDepartment of Electrical Engineering, Princeton University 32 , Princeton, New Jersey 08544, USABarry P. RandAndlinger Center for Energy and the Environment, Princeton University 33 , Princeton, New Jersey 08544, USANadja GlückDepartment of Chemistry, Ludwig-Maximilians-University Munich 34 , Butenandtstr. 5-13, 81377 Munich, GermanyThomas BeinDepartment of Chemistry, Ludwig-Maximilians-University Munich 34 , Butenandtstr. 5-13, 81377 Munich, GermanyFabio MatteocciCHOSE—Centre for Hybrid and Organic Solar Energy, Department of Electronic Engineering, University of Rome Tor 35 Vergata, Roma 00133, ItalyLuigi Angelo CastriottaCHOSE—Centre for Hybrid and Organic Solar Energy, Department of Electronic Engineering, University of Rome Tor 35 Vergata, Roma 00133, ItalyAldo Di CarloCHOSE—Centre for Hybrid and Organic Solar Energy, Department of Electronic Engineering, University of Rome Tor 35 Vergata, Roma 00133, ItalyMatthias SchefflerFritz-Haber-Institut der Max-Planck-Gesellschaft 38 , Faradayweg 4-6, 14195 Berlin, GermanyClaudia DraxlFritz-Haber-Institut der Max-Planck-Gesellschaft 38 , Faradayweg 4-6, 14195 Berlin, Germany
2021en
ABI

Annotatsiya

Metal halide perovskites are the first solution processed semiconductors that can compete in their functionality with conventional semiconductors, such as silicon. Over the past several years, perovskite semiconductors have reported breakthroughs in various optoelectronic devices, such as solar cells, photodetectors, light emitting and memory devices, and so on. Until now, perovskite semiconductors face challenges regarding their stability, reproducibility, and toxicity. In this Roadmap, we combine the expertise of chemistry, physics, and device engineering from leading experts in the perovskite research community to focus on the fundamental material properties, the fabrication methods, characterization and photophysical properties, perovskite devices, and current challenges in this field. We develop a comprehensive overview of the current state-of-the-art and offer readers an informed perspective of where this field is heading and what challenges we have to overcome to get to successful commercialization.

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