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Low-temperature processed meso-superstructured to thin-film perovskite solar cells

James M. BallDepartment of Physics, University of Oxford, Clarendon Laboratory, Parks Road, Oxford, UKMichael M. LeeDepartment of Physics, University of Oxford, Clarendon Laboratory, Parks Road, Oxford, UKAndrew HeyDepartment of Physics, University of Oxford, Clarendon Laboratory, Parks Road, Oxford, UKHenry J. SnaithDepartment of Physics, University of Oxford, Clarendon Laboratory, Parks Road, Oxford, UK
2013en
ABI

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We have reduced the processing temperature of the bulk absorber layer in CH3NH3PbI3−xClx perovskite solar cells from 500 to <150 °C and achieved power conversion efficiencies up to 12.3%. Remarkably, we find that devices with planar thin-film architecture, where the ambipolar perovskite transports both holes and electrons, convert the absorbed photons into collected charge with close to 100% efficiency.

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