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Color-selective semiconductor nanocrystal laser

Hans‐Jürgen EislerDepartment of Chemistry and Center for Materials Science and Engineering, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge Massachusetts 02139Vikram SundarDepartment of Chemistry and Center for Materials Science and Engineering, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge Massachusetts 02139Moungi G. BawendiDepartment of Chemistry and Center for Materials Science and Engineering, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge Massachusetts 02139Michael WalshNanostructures Laboratory, Department of Electrical Engineering and Computer Science, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge Massachusetts 02139Henry I. SmithNanostructures Laboratory, Department of Electrical Engineering and Computer Science, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge Massachusetts 02139Victor I. KlimovChemistry Division, C-PCS, Los Alamos National Laboratories, Los Alamos, New Mexico 87545
2002en
ABI

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Theoretical predictions of the benefits of three-dimensional quantum confinement have provided motivation for the development of quantum-dot lasers. Such lasers, developed in the case of self-assembled quantum dots, have not been successfully demonstrated with quantum-confined colloidal nanocrystals (NCs). Here, using recently developed NC-titania chemistry, we report the successful development of an optically pumped, NC-based distributed feedback laser, in which the narrow gain profiles of these nanoparticles have been matched with the feedback of a second-order distributed feedback laser. This laser, whose output color can be selected by choosing appropriately sized nanocrystals, operates at 80 K and at room temperature.

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