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Large scale electrochemical synthesis of high quality carbon nanodots and their photocatalytic property

Hai MingInstitute of Functional Nano & Soft Materials (FUNSOM) and Jiangsu Key Laboratory for Carbon Based Functional Materials & Devices, Soochow University, Suzhou, Jiangsu 215123, People's Republic of ChinaZheng MaInstitute of Functional Nano & Soft Materials (FUNSOM) and Jiangsu Key Laboratory for Carbon Based Functional Materials & Devices, Soochow University, Suzhou, Jiangsu 215123, People's Republic of ChinaYang LiuInstitute of Functional Nano & Soft Materials (FUNSOM) and Jiangsu Key Laboratory for Carbon Based Functional Materials & Devices, Soochow University, Suzhou, Jiangsu 215123, People's Republic of ChinaKeming PanInstitute of Functional Nano & Soft Materials (FUNSOM) and Jiangsu Key Laboratory for Carbon Based Functional Materials & Devices, Soochow University, Suzhou, Jiangsu 215123, People's Republic of ChinaHang YuInstitute of Functional Nano & Soft Materials (FUNSOM) and Jiangsu Key Laboratory for Carbon Based Functional Materials & Devices, Soochow University, Suzhou, Jiangsu 215123, People's Republic of ChinaFang WangInstitute of Functional Nano & Soft Materials (FUNSOM) and Jiangsu Key Laboratory for Carbon Based Functional Materials & Devices, Soochow University, Suzhou, Jiangsu 215123, People's Republic of ChinaZhenhui KangInstitute of Functional Nano & Soft Materials (FUNSOM) and Jiangsu Key Laboratory for Carbon Based Functional Materials & Devices, Soochow University, Suzhou, Jiangsu 215123, People's Republic of China
2012en
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High quality carbon nanodots (C-dots) with high purity were synthesized through a mild, one-step electrochemical approach, without the assistance of any chemicals but only pure water. This high productivity method makes the synthetic process of C-dots synthesis both economical as well as environment-friendly. The as prepared C-dots are predominantly multi-layer graphene oxide, with luminescence and high up-conversion photoluminescence (emission of light at shorter wavelengths than the excitation wavelength). Meanwhile, C-dots showed peroxidise mimetic function and visible-light-sensitive photocatalytic activity for methyl orange degradation. In addition, a novel photocatalyst (TiO(2)/C-dots) was obtained by combining C-dots with TiO(2) through an easy hydrothermal method. Remarkably, TiO(2)/C-dots exhibited an excellent visible-light photocatalytic activity.

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