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Interplay between the magnetic and transport properties in the III-V diluted magnetic semiconductor<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">Ga</mml:mi></mml:mrow><mml:mrow><mml:mn>1</mml:mn><mml:mi>−</mml:mi><mml:mi>x</mml:mi></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">Mn</mml:mi></mml:mrow><mml:mrow><mml:mi>x</mml:mi></mml:mrow></mml:msub></mml:mrow><mml:mi mathvariant="normal">As</mml:mi></mml:math>

A. Van EschIMEC, Kapeldreef 75, B-3001 Leuven, BelgiumL. Van BockstalLaboratorium voor Vaste-Stoffysica en Magnetisme, Katholieke Universiteit Leuven, B-3001 Leuven, BelgiumJ. De BoeckIMEC, Kapeldreef 75, B-3001 Leuven, BelgiumG. VerbanckLaboratorium voor Vaste-Stoffysica en Magnetisme, Katholieke Universiteit Leuven, B-3001 Leuven, BelgiumA. S. van SteenbergenResearch Institute for Materials, High Field Magnet Laboratory, University of Nijmegen, 6525 ED Nijmegen, The NetherlandsPeter J. WellmannMaterials Department, University of California, Santa Barbara, California 93106B. GrietensIMEC, Kapeldreef 75, B-3001 Leuven, BelgiumRia BogaertsLaboratorium voor Vaste-Stoffysica en Magnetisme, Katholieke Universiteit Leuven, B-3001 Leuven, BelgiumF. HerlachLaboratorium voor Vaste-Stoffysica en Magnetisme, Katholieke Universiteit Leuven, B-3001 Leuven, BelgiumG. BorghsIMEC, Kapeldreef 75, B-3001 Leuven, Belgium
1997lv
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Using a low-temperature molecular-beam epitaxy growth procedure, ${\mathrm{Ga}}_{1\ensuremath{-}x}{\mathrm{Mn}}_{x}\mathrm{As}$ --- a III-V diluted magnetic semiconductor --- is obtained with Mn concentrations up to $x\ensuremath{\sim}9%.$ At a critical temperature ${T}_{c}$ (${T}_{c}\ensuremath{\approx}50\mathrm{K}$ for $x=0.03--0.05$), a paramagnetic to ferromagnetic phase transition occurs as the result of the interaction between $\mathrm{M}\mathrm{n}\ensuremath{-}h$ complexes. Hole transport in these compounds is strongly affected by the antiferromagnetic exchange interaction between holes and Mn $3d$ spins. A model for the transport behavior both above and below ${T}_{c}$ is given. Above ${T}_{c},$ all materials exhibit transport behavior which is characteristic for systems near the metal-insulator transition. Below ${T}_{c},$ due to the rising spontaneous magnetization, spin-disorder scattering decreases and the relative position of the Fermi level towards the mobility edge changes. When the magnetization has reached its saturation value (below $\ensuremath{\sim}10\mathrm{K}$) variable-range hopping is the main conduction mechanism. The negative magnetoresistance is the result of the expansion of the hole wave functions in an applied magnetic field.

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