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Transmutation of long-lived fission products in an advanced nuclear energy system

Xiaobo SunSchool of Nuclear Science and Technology, University of South China, Hengyang, 421001, ChinaWen LuoSchool of Nuclear Science and Technology, University of South China, Hengyang, 421001, China. [email protected]Haoyang LanSchool of Nuclear Science and Technology, University of South China, Hengyang, 421001, ChinaYingming SongSchool of Nuclear Science and Technology, University of South China, Hengyang, 421001, ChinaQingyu GaoInstitute of Modern Physics, Chinese Academy of Sciences, Lanzhou, 730000, ChinaZhichao ZhuSchool of Nuclear Science and Technology, University of South China, Hengyang, 421001, ChinaJ. G. ChenShanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai, 201800, China. [email protected]X. Z. CaiShanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai, 201800, China

2022en

ABI

Annotatsiya

Abstract Disposal of long-lived fission products (LLFPs) produced in reactors has been paid a lot attention for sustainable and clean nuclear energy. Although a few transmutation means have been proposed to address this issue, there are still scientific and/or engineering challenges to achieve efficient transmutation of LLFPs. In this study, we propose a novel concept of advanced nuclear energy system (ANES) for transmuting LLFPs efficiently without isotopic separation. The ANES comprises intense photoneutron source (PNS) and subcritical reactor, which consist of lead–bismuth (Pb-Bi) layer, beryllium (Be) layer, and fuel, LLFPs and shield assemblies. The PNS is produced by bombarding radioactive cesium and iodine target with a laser-Compton scattering (LCS) γ-ray beam. We investigate the effect of the ANES system layout on transmutation efficiency by Monte Carlo simulations. It is found that a proper combination of the Pb-Bi layer and the Be layer can increase the utilization efficiency of the PNS by a factor of ~ 10, which helps to decrease by almost the same factor the LCS γ-beam intensity required for driving the ANES. Supposing that the ANES operates over 20 years at a normal thermal power of 500 MWt, five LLFPs including 99 Tc, 129 I, 107 Pd, 137 Cs and 79 Se could be transmuted by more than 30%. Their effective half-lives thus decrease drastically from ~ 10 6 to less than 10 2 years. It is suggested that this successful implementation of the ANES paves the avenue towards practical transmutation of LLFPs without isotopic separation.

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DOI: 10.1038/s41598-022-06344-y

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