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Discontinuous atmospheric pressure interface for mass spectrometry using a solenoid pulse valve

Dilshadbek T. UsmanovClean Energy Research Center University of Yamanashi Takeda‐4, Kofu Yamanashi 400‐8511 JapanKenzo HiraokaClean Energy Research Center University of Yamanashi Takeda‐4, Kofu Yamanashi 400‐8511 Japan
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Abstract

RATIONALE: For the development of on-site mass spectrometry for security and safety, point-of-care analysis, etc., the gas volume introduced into the vacuum should be reduced to a minimum. To cope with this demand, a discontinuous atmospheric pressure interface using a solenoid pulse valve was developed. METHODS: The sample gas was introduced discontinuously into the ionization cell with a volume of 0.17 cm(3) . The sampled gas in the cell was ionized by an alternating current (ac) corona discharge. The generated ions were sampled through a 0.25 mm i.d. and 12 mm long nickel capillary into the vacuum of a time-of-flight mass spectrometer. RESULTS: A gas flow rate of ~25 mL/min was achieved with the 1 Hz pulse valve operation and 20 ms valve opening time. Sub-ng limits of detection for less volatile compounds such as explosives and drugs were obtained. CONCLUSIONS: Due to its compact size and low gas load to the vacuum, this new interface may be useful for applications in miniaturized mass spectrometry. Copyright © 2016 John Wiley & Sons, Ltd.

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