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Influence of C60 morphology on high-order harmonic generation enhancement in fullerene-containing plasma

R. A. GaneevRaja Ramanna Centre for Advanced Technology 1 , Indore 452013, IndiaH. SinghalRaja Ramanna Centre for Advanced Technology 1 , Indore 452013, IndiaP. A. NaikRaja Ramanna Centre for Advanced Technology 1 , Indore 452013, IndiaJ. A. ChakeraRaja Ramanna Centre for Advanced Technology 1 , Indore 452013, IndiaArvind K. SrivastavaRaja Ramanna Centre for Advanced Technology 1 , Indore 452013, IndiaT. S. DhamiRaja Ramanna Centre for Advanced Technology 1 , Indore 452013, IndiaM. P. JoshiRaja Ramanna Centre for Advanced Technology 1 , Indore 452013, IndiaP. D. GuptaRaja Ramanna Centre for Advanced Technology 1 , Indore 452013, India
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The morphologies of the fullerene targets and the ablated fullerenes to determine the optimal conditions of excitation of the C60-containing targets have been analyzed. The optimization of fullerene-containing plasma conditions allowed the enhanced harmonic generation in these plasmas using laser radiation of different wavelengths, pulse durations, and phase modulation. A comparison between the harmonic generation in single-atom/ion-containing plasmas (using bulk carbon, silver, and indium targets) and fullerene-rich plasma plumes showed better conversion efficiency for the latter medium. The influence of phase modulation of the fundamental radiation in fullerene plasmas on the spectral properties of harmonics has been studied.

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